Laser cooling and trapping of atoms: beyond the limits
Transcription
Laser cooling and trapping of atoms: beyond the limits
Laser cooling and trapping of atoms: beyond the limits 1. A breakthrough in the quest of 4. Dipolar force 1. Properties; interpretations low temperatures 2. Applications: optical tweezer 2. Radiative forces optical lattice, atomic mirror 1. Semi classical approach 3. Photon momentum 2. Atomic motion interpretation? 3. Radiative forces 5. Laser cooling: optical molasses 4. Resonance transition 1. Doppler cooling 3. Resonant radiation pressure 2. Magneto Optical Trapp (MOT) 1. Properties 3. Doppler Limit temperature 2. Stopping a laser beam 4. Below Doppler limit: Sisyphus with radiation pressure 6. Below the one photon recoil limit: 3. Photon momentum dark resonance cooling and Lévy interpretation flights 1 Laser cooling of atoms: a breakthrough 1 cm/s − 10 9 K − 10 6 K 1 m/s 300 m/s − 10 3 K 1K Dilution cryostats Sub recoil cooling 1988 Sisyphus 1988 Doppler molasses 1985 103 K room Liquid He 1908 L’échelle logarithmique montre l’ampleur du refroidissement, caractérisée par une division de la température absolue, pas par une soustraction. 2 Cooling and trapping: increase of phase space density Cooling: • Increase of density in velocity space • ≠ filtering Trapping : • Confinement in real space Cooling and Trapping : • Increase of phase space density 3 Laser cooling and trapping of atoms: beyond the limits 1. A breakthrough in the quest of 4. Dipolar force 1. Properties; interpretations low temperatures 2. Applications: optical tweezer 2. Radiative forces optical lattice, atomic mirror 1. Semi classical approach 3. Photon momentum 2. Atomic motion interpretation? 3. Radiative forces 5. Laser cooling: optical molasses 4. Resonance transition 1. Doppler cooling 3. Resonant radiation pressure 2. Magneto Optical Trapp (MOT) 1. Properties 3. Doppler Limit temperature 2. Stopping a laser beam 4. Below Doppler limit: Sisyphus with radiation pressure 6. Below the one photon recoil limit: 3. Photon momentum dark resonance cooling and Lévy interpretation flights 4 Semi classical model of atom-light interaction Matter (atoms) is quantized Light described by classical electromagnetic field Successful to describe all matter-light interaction phenomenon known until 1970 (except spontaneous emission) • Absorption, stimulated emission: lasers • Photoelectric effect!!! Modern quantum optics is about radiation that demand quantization of light • Single photon wave packets • Entangled photons Semi-classical model is very useful, provided one knows its limits 5 Two level atom in motion: quantum description Etat interne ψ ∈ Eint (dimension 2) ⎡γ a (t ) ⎤ ψ ↔⎢ ⎥ γ ( t ) ⎣ b ⎦ Eb =ω 0 Ea ⎡0 0 ⎤ ˆ H0 = ⎢ ⎥ ω = 0 0⎦ ⎣ Mouvement du centre de masse (observables r , P ) ψ ∈ Er ψ ↔ ψ (r , t ) Hˆ ext 2 Pˆ 2 = = ↔ Hˆ ext = − Δ 2M 2M ↔ spineur Description globale ψ ∈ Eint ⊗ Er ⎡ψ a (r, t ) ⎤ ψ ↔⎢ ⎥ ⎣ψ b (r, t ) ⎦ Hˆ = Hˆ 0 + Hˆ ext Description quantique de la dynamique interne et du mouvement 6 Interaction avec une onde électromagnétique classique G Interaction dipolaire électrique avec E(r, t ) = ε E0 (r ) cos (ω t − ϕ (r ) ) ⎡0 ˆ ˆ ˆ H I = − D ⋅ E = − Dε Eε (r, t ) = − ⎢ ⎣d G d⎤ ˆ ˆ Eε (r, t ) avec Dε = D ⋅ ε ⎥ 0⎦ ˆ2 0 0 ⎡ ⎤ ⎡ 0 dε ⎤ P ˆ ˆ ˆ ˆ H = H 0 + H ext + H I = ⎢ Eε (r, t ) + Δ−⎢ ⎥ ⎥ ⎣0 =ω 0 ⎦ 2 M ⎣ dε 0 ⎦ ⎡ψ a (r, t ) ⎤ Agit sur [ψ ] = ⎢ ⎥ t γ r ( , ) ⎣ b ⎦ L’hamiltonien dipolaire électrique est valable dans le cadre de l’approximation des grandes longueurs d’onde: distance électronnoyau << λ Cela ne met aucune contrainte sur ψa(r,t) et ψb(r,t) qui pourraient être étalés sur une distance >> λ 7 Paquet d’onde localisé: limite classique Atome localisé Paquet d’onde étroit, identique pour les deux états ⎡ψ a (r, t ) ⎤ ⎡γ a (t ) ⎤ ψ (r , t ) =⎢ [ψ ] = ⎢ ⎥ ⎥ ⎣ γ b ( r , t ) ⎦ ⎣γ b ( t ) ⎦ ψ (r, t ) « piqué » autour de rat largeur << λ Position classique rˆ (t ) = ψ rˆ ψ = ∫ψ * (r, t ) rψ (r, t ) d 3 r rat (t ) Vitesse classique définie par Th. d’Ehrenfest: ˆ d 1 P ⎡rˆ , Hˆ ⎤ = Vat = rˆ = ⎦ dt i= ⎣ M d d Vat = rat (t ) = rˆ (t ) dt dt ⎡ Pˆ 2 ⎤ Pˆ Pˆ ˆ ⎡rˆ , P ⎤ = car ⎢rˆ , i= ⎥ =2 ⎣ ⎦ 2 M 2 M M ⎣ ⎦ 8 Dynamique de la position classique ˆ drat P On applique le th. d’Ehrenfest à la vitesse classique = Vat = dt M d 1 ˆ ˆ 1 ˆ ˆ ⎡ P, H ⎤ = ⎡ P, H I ⎤ M Vat = ⎣ ⎦ ⎦ dt i= i= ⎣ = ˆ G ˆ ˆ ˆ ˆ ⎡ P, H I ⎤ = − Dε ⎡ P, E (r, t ) ⎤ = − Dε ∇ {E (r, t )} ⎣ ⎦ ⎣ ⎦ i G G d2 d ˆ ˆ M 2 rat = M Vat = Dε ∇ { E (r, t )} = Dε ⎡⎣∇ { Eε (r, t )}⎤⎦ rat dt dt L’atome suit une trajectoire classique moyenne déterminée par la force G ˆ F = Dε ⎡⎣∇ { Eε (r, t )}⎤⎦ rat G E = ε Eε (r, t ) cf. électrodynamique classique, pour un dipôle dε dans G G F = dε ∇Eε (et pas ∇( dε Eε ): important quand dε dépend de Eε ) 9 Forces radiatives Oscillation forcée du dipôle atomique, sous l’effet du champ G G E(r, t ) = ε E0 (r ) cos (ω t − ϕ (r ) ) = ε E (r, t ) + c.c. avec E (r, t ) = E0 (r ) 2 exp {iϕ (r )}exp {−iω t} Dˆ ε = ε 0α E (r, t ) + ε 0α *E *(r, t ) après amortissement du transitoire Polarisabilité complexe α = α ′ + iα ′′ (cf. chap II) Force due à l’interaction entre le champ et le dipôle atomique induit G G * * ˆ F = Dε ⎡⎣∇ {E (r, t )}⎤⎦ = ε 0 (α E + α E ) ∇ {E + E * } rat En ne gardant que les termes qui n’oscillent pas (moyenne temporelle) G * F = ε 0α E ⎡⎣∇E ⎤⎦ + c.c. rat 10 Radiation pressure vs Dipole force G * F = ε 0α E ⎡⎣∇E ⎤⎦ α = α ′ + iα ′′ rat + c.c. F= avec E (r, t ) = ε 0α 4 E0 (r ) 2 exp {iϕ (r )}exp {−iω t} G G E0 (r ) ∇ [ E0 (r ) ] − i∇ [ϕ (r ) ] E0 (r ) + c.c. ( ) G ε 0α ′′ 2 G = E0 (r )∇ [ E0 (r ) ] + ( E0 (r ) ) ∇ [ϕ (r )] 2 2 l’expression étant évaluée en r = rat ε 0α ′ G • Partie réactive (réelle) de la Fdip = E0 (r)∇[ E0 (r)] Force dipolaire polarisabilité 2 ε0α′ • Gradient de l’amplitude ε0α′′ 2 G Fres = ( E0 (r)) ∇[ϕ(r)] 2 Pression de radiation résonnante • Partie dissipative (imaginaire) de la polarisabilité • Gradient de la phase 11 Closed two level transition (resonance line) Raie « de résonance »: niveau du bas fondamental ¾ Durée de vie infinie Γa = 0 =ω 0 =ω Γ ¾ Largeur de raie Γ = Γb Ea ¾ Transition fermée G G Dipôle forcé sous l’effet de E = ε E0 cos (ω t − ϕ ) = ε E + E * Eb ( ) Utilisation du formalisme de la matrice densité et des équations de Bloch optiques (dissipation, cf. Maj. 2) G Dˆ ε = ε 0α E + ε 0α *E *(r, t ) D = ε D̂ε =Ω = − d E 1 ⎡0 d ⎤ Dˆ ε = − ⎢ ⎥ 0 d ⎣ ⎦ 15 d2 1 1 α= ε 0 = (ω − ω ) − i Γ 1 + s 0 2 Réponse linéaire 0 Ω12 / 2 s= (ω 0 − ω ) 2 + Γ 2 / 4 saturation 12 Laser cooling and trapping of atoms: beyond the limits 1. A breakthrough in the quest of 4. Dipolar force 1. Properties; interpretations low temperatures 2. Applications: optical tweezer 2. Radiative forces optical lattice, atomic mirror 1. Semi classical approach 3. Photon momentum 2. Atomic motion interpretation? 3. Radiative forces 5. Laser cooling: optical molasses 4. Resonance transition 1. Doppler cooling 3. Resonant radiation pressure 2. Magneto Optical Trapp (MOT) 1. Properties 3. Doppler Limit temperature 2. Stopping a laser beam 4. Below Doppler limit: Sisyphus with radiation pressure 6. Below the one photon recoil limit: 3. Photon momentum dark resonance cooling and Lévy interpretation flights 13 Pression de radiation résonnante Onde plane progressive E0 exp {ik ⋅ r}exp {−iω t} 2 G ε 0α ′ = E0 (r )∇ [ E0 (r ) ] = 0 2 E (r , t ) = amplitude E0 constante ⇒ Fdip G d 2 E0 2 Γ/2 1 E ( ) ( ) Fres = r ∇ ϕ r = k ( 0 ) [ ] 2 2= (ω 0 − ω ) 2 + Γ 2 / 4 1 + s ε 0α ′′ 2 Ω12 Γ/2 1 Γ s Fres ==k = =k 2 2 2 (ω 0 − ω ) + Γ / 4 1 + s 2 1+ s Ω12 / 2 I 1 s= = (ω 0 − ω ) 2 + Γ 2 / 4 I sat 1 + 4(ω 0 − ω ) 2 / Γ 2 paramètre de saturation 14 Resonant radiation pressure: properties Fres ==k Γ s 2 1+ s • Dirigée suivant le vecteur d’onde du laser Fres k Fres Ω12 / 2 Γ Fres ==k 2 (ω 0 − ω ) 2 + Ω12 / 2 + Γ 2 / 4 Fmax • Lorentzian resonance (power broadening) Ω12 / 2 I • Saturation s0 = 2 = Γ / 4 I sat Γ s0 Fmax = =k 2 1 + s0 =k Γ 2 ω0 1 1 s ω Order of magnitude ⎧ Γ / 2π = 6 MHz Rb ⎨ 2 I = 1.6 mW / cm ⎩ sat Fmax Γ 1 + s0 =k = 5.9 ×10−3 m / s M max Fmax =k Γ = ≈ 105 m / s −2 ≈ 104 g M M 2 Easily achievable with lasers 15 Decelerating atoms with radiation pressure Jet thermique de sodium V≈ 2 k BT ≈ 600 m / s M V 2 36 × 104 ≈ = 1.8 m distance d'arret = 5 2γ 2 × 10 Challenges (Phillips, 2002): keep atoms on resonance during deceleration (Doppler effect changes); avoid optical pumping into other levels Ralentissement « Zeeman » (Phillips et coll., 1982) Distribution des vitesses Densité dans l’espace des vitesses augmente: vrai refroidissement Full stop achieved in 1985 16 Stopping metastable Helium atoms 17 Radiation pressure and fluorescence rate Pression de radiation résonnante Γ s Fres ==k 2 1+ s Rfluo = Γ s 2 1+ s E0 E (r , t ) = exp {ik ⋅ r}exp {−iω t} 2 Ω12 / 2 s= (ω 0 − ω ) 2 + Γ 2 / 4 =Ω1 = − d ⋅ E0 Eb Fres ==kRfluo =ω 0 = ω Γ Taux de fluorescence (nombre de cycles par seconde, calcul par EBO) Cycle de fluorescence: Un photon du faisceau incident est diffusé dans une direction différente, avec une énergie égale (diffusion élastique) ou un peu différente (diffusion inélastique) Ea k,ω k sp , ωsp ksp : direction aléatoire Réinterprétation de la pression de radiation résonnante ? 18 Radiation pressure and photon momentum Bilan d’impulsion dans un cycle de fluorescence (diffusion d’un photon) Photon dans une onde plane Eb =k sp de vecteur d’onde k : p = =k =k =k =k =k sp Absorption-Réémission − =k sp ΔPat = =k − =k sp ΔPat Ea Moyenné sur un grand nombre de cycles k sp = 0 ⇒ ΔPat 1 cycle = =k Force moyenne Fres =Rfluo ΔPat 1 cycle Γ s = Rfluo =k = =k 2 1+ s Modèle tout quantique (photons): calcul plus simple, image plus simple, même résultat ! De plus, suggère l’existence de fluctuations de la force liées aux fluctuations de la direction d’émission. 19 The problem of many ground state levels: avoiding optical depumping Alkali atoms have an hyperfine structure Ground state is split in many components Optical pumping into non interacting levels leads to deceleration stopping. Take advantage of selection rules (choice of polarization) Use repumping lasers 20 Laser cooling and trapping of atoms: beyond the limits 1. A breakthrough in the quest of 4. Dipolar force 1. Properties; interpretations low temperatures 2. Applications: optical tweezer 2. Radiative forces optical lattice, atomic mirror 1. Semi classical approach 3. Photon momentum 2. Atomic motion interpretation? 3. Radiative forces 5. Laser cooling: optical molasses 4. Resonance transition 1. Doppler cooling 3. Resonant radiation pressure 2. Magneto Optical Trapp (MOT) 1. Properties 3. Doppler Limit temperature 2. Stopping a laser beam 4. Below Doppler limit: Sisyphus with radiation pressure 6. Below the one photon recoil limit: 3. Photon momentum dark resonance cooling and Lévy interpretation flights 21 Force dipolaire Fdip = ε 0α ′ 2 G E0 (r )∇ [ E0 (r ) ] 2 d = = Fdip 2 exp {iϕ (r )} exp {−iω t} G ≠ 0 pour une onde inhomogène : ∇E0 ≠ 0 Fdip Fdip avec E (r, t ) = E0 ( r ) G 2 ∇ [ E0 (r )] ω0 − ω (ω 0 − ω ) 2 + Γ 2 G =(ω 0 − ω ) ∇ [ s (r )] = 1 + s (r ) 2 1 + s (r ) 4 G =(ω − ω 0 ) = − ∇ [U (r ) ] avec U (r ) = log [1 + s (r ) ] 2 1 Dérive d’un potentiel (partie réactive de la s (r ) = I (r ) 2 2 + ω − ω Γ 1 4( ) / I sat 0 polarisabilité) variant comme l’intensité Applications ⎧ attiré vers haute intensité si ω < ω 0 atome ⎨ ⎩repoussé par haute intensité si ω > ω 0 22 An optical trap: optical tweezer I (r ) 1 =(ω − ω 0 ) r = avec s ( ) U dip (r ) = log [1 + s (r )] 2 2 + ω − ω Γ I 1 4( ) / sat 0 2 Trapping by a focused laser beam with ω < ω0 : optical tweezer laser Shallow trap: demands very cold atoms ( T < 1 mK ) Classical interpretation: coupling of the field with the induced dipole Interpretation by light shifts of the atomic levels (Cohen-Tannoudji, Dalibard): Atom spends more time in ground state. Case of large detuning: atom in g: no fluctuation, but very shallow, ultra cold atoms e ω L < ω0 g 23 Manipulation d’atomes individuels (P. Grangier) 2 atomes côte à côte Piégeage intermittent d’un seul atome 24 Piège dipolaire: réseau optique Piégeage aux ventres (ω < ω0) ou aux nœuds (ω > ω0) d’une onde stationnaire 3 dimensions: potentiel dipolaire cf. G. Grynberg et coll. Atomes dans les micro puits 25 Miroir atomique à ondes évanescentes ccd sonde Onde évanescente 5 cm Atomes froids (100 μK) lâchés depuis un piège Atomes repoussés (ω > ω0 : barrière de potentiel) quand ils entrent dans l’onde évanescente : rebond 26 Dipole force and photon momentum Onde inhomogène = plusieurs ondes planes • Absorption de =k1 • Emission stimulée de =k2 =k1 ΔPat = =k1 − =k 2 =k 2 Eb − =k 2 =k1 ΔPat Mais on doit aussi considérer: • Absorption de =k2 • Emission stimulée de =k1 =k1 =k 2 Ea Force de signe opposé !!?? La phase relative des ondes 1 et 2 détermine quel processus domine. • Délicat dans le modèle tout quantique (photons) • Automatiquement pris en compte dans le modèle classique du champ (la phase relative détermine le gradient d’intensité) 27 Laser cooling and trapping of atoms: beyond the limits 1. A breakthrough in the quest of 4. Dipolar force 1. Properties; interpretations low temperatures 2. Applications: optical tweezer 2. Radiative forces optical lattice, atomic mirror 1. Semi classical approach 3. Photon momentum 2. Atomic motion interpretation? 3. Radiative forces 5. Laser cooling: optical molasses 4. Resonance transition 1. Doppler cooling 3. Resonant radiation pressure 2. Magneto Optical Trapp (MOT) 1. Properties 3. Limit temperature of Doppler c. 2. Stopping a laser beam 4. Below Doppler limit: Sisyphus with radiation pressure 6. Below the one photon recoil limit: 3. Photon momentum dark resonance cooling and Lévy interpretation flights 28 Refroidissement Doppler Pression de radiation par deux ondes opposées k,ω −k , ω Vat ω < ω0 Lasers non saturants, désaccordés sous la résonance Eb =ω 0 = ω Γ Ea Vitesse atomique: effet Doppler différent pour les deux ondes ⎧ ⎫ Γ2 / 4 Γ2 / 4 Fres =F0 ⎨ − ⎬ 2 2 2 2 ⎩ (ω − k ⋅ Vat − ω 0 ) + Γ / 4 (ω + k ⋅ Vat − ω 0 ) + Γ / 4 ⎭ F ω0 − ω k ω = ω0 − Γ 2 Vat Force opposée à la vitesse: freinage ⇒ refroidissement Généralisable à 3 dimensions 29 Mélasse Doppler Autour de V = 0 : frottement visqueux dV F = −α M V ou = −αV dt k,ω F ω0 − ω =k 2 Γ α= s0 pour ω = ω 0 − 2 M Ordre de grandeur (rubidium, s0 = 0.5) α 2.5 ×10−4 s −1 −k , ω Vat k ω = ω0 − Vat Γ 2 Temps d’amortissement : 40 μs ! Milieu très visqueux: « mélasse optique » Refroidissement exponentiel ! atomes « englués » d 2 V = −2α V 2 dt La température décroît : jusqu’où ? Sous le mK ! 30 Magneto Optical Trap: molasses with a restoring force Zeeman differential detuning and polarized lasers ω < ω0 Je = 1 −k , ω k,ω m = −1 m = 0 B σ− σ+ B σ− z m =1 σ+ g z Quadrupole magnetic field: sign changes at z = 0 Jg = 0 Bz < 0 : σ− polarized beam more efficient than σ+ Atom pushed towards z = 0: trapping. Doppler molasses also at work. ⇒ Overdamped trap. Works in 3D . “The work horse of cold atoms” 31 What is the limit temperature in doppler molasses of Magneto Optical trap? We have a cooling process that never stops. Is there a heating process? 32 Heating: fluctuations of radiative forces Semi-classical approach G ˆ F = Dε ⎡⎣∇ { E (r, t )}⎤⎦ rat D : quantum average, over an ensemble of atoms, submitted to the same radiation. Many atoms: a genuine ensemble! Each atom is submitted to a different force F , whose average is F. G G2 F (t ) = F (t ) F (t ) − F 2 (t ) = ΔF 2 V V ΔV 2 / ⇒ Velocity dispersion ⇒ heating increases with time t Heating due to the quantum character of atomic dipole. There is another point of view, based on momentum exchanges with photons 33 Fluctuations of radiation pressure: a photon point of view At each fluorescence cycle, there is a spontaneous emission random recoil which is not taken into account in the average force =k sp =k L =k L ΔPat 2DP = ( =k ) Rfluo 2 Random walk in the atom momentum space: step =k , rate Rfluo d 2 P = 2D dt Diffusion coefficient (Einstein) Heating 34 Limit of Doppler cooling d 2 P = −2α P 2 dt Cooling d 2 P = 2D dt Heating Steady state Pat 2 Can be described with a Langevin equation = D α Relation d’Einstein G d Pat = −α Pat + Fchauff dt Température finale Pat 3 3 = =Γ kBT = 2 2M 4 2 Ordre de grandeur : 100 μK Demonstrated in 1985 (S. Chu) 35 Below the Doppler limit: Sisyphus cooling Doppler limit: 100 μK range (observed in 1985, S. Chu) 1988: limit temperature found in the 10 μK range, well below the “theroretical” limit of Doppler cooling (WD Phillips) Interprétation (C. Cohen-Tannoudji, J. Dalibard): “Sisyphus effect”. Must take into account ground state degeneracy, and light polarization gradients that one cannot avoid in a 3D standing wave. Because of delay to reach internal steady state (motion) the atom tends to spends more time climbing hills than descending: looses kinetic energy. Residual velocity: a few recoil velocity VR = =k M Ultimate limit? 36 Laser cooling and trapping of atoms: beyond the limits 1. A breakthrough in the quest of 4. Dipolar force 1. Properties; interpretations low temperatures 2. Applications: optical tweezer 2. Radiative forces optical lattice, atomic mirror 1. Semi classical approach 3. Photon momentum 2. Atomic motion interpretation? 3. Radiative forces 5. Laser cooling: optical molasses 4. Resonance transition 1. Doppler cooling 3. Resonant radiation pressure 2. Magneto Optical Trapp (MOT) 1. Properties 3. Doppler Limit temperature 2. Stopping a laser beam 4. Below Doppler limit: Sisyphus with radiation pressure 6. Below the one photon recoil limit: 3. Photon momentum dark resonance cooling and Lévy interpretation flights 37 The one photon recoil: an ultimate limit? 1 cm/s − 10 9 K 1 m/s − 10 6 K 300 m/s − 10 3 K 1K 103 K subrecoil liquid He Sisyphus room Doppler molasses Experiments show that ultimate limit of Sisyphus corresponds to a few single photon recoil =k ) 3 ( kBT ≈ 10 2 2M 2 In agreement with the concept that spontaneous emission is necessary (dissipation, non hamiltonian), and cannot be controlled. 38 Below the recoil limit: velocity selective coherent population trapping (“dark resonance cooling”) 1988 (ENS Paris; CCT, AA): demonstration of a method allowing one to obtain a gas with velocity distribution narrower than the recoil velocity associated with the emission or absorption of a single photon V R = = k M Necessary to use a quantum description of the atomic motion New theoretical approaches: • Quantum Monte-Carlo; delay function • Lévy flights statistics See “special” (vintage) seminar 39 Laser cooling and trapping of atoms: a fantastic new tool In less than one decade (1980’s), it has been possible to reach goals that were thought to be very far ahead: • Cooling atoms in the μK range • Trapping atoms and keeping them for seconds Experimental surprises as well as ingenuity has allowed physicits to break several so called “limits”, and prompted them to revisit atomlight interaction. This new tool for atomic physics has paved the way to gaseous Bose Einstein Condensates and the many recent developments at the frontier between Condensed Matter Physics and Atomic Molecular and Optical Physics 40